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Certain places felt spiritual, the Golden Dome, Temples etc, mind you, the Wailing wall didn't, just touristy, but thats the same anywhere,
I think its because in these places, its always quiet, and people move about in them in a hushed respectful way, and you are, because your there, infected with the same, also, you don't want to offend.
As to Israel itself, no, not spiritual, but the people there have a fatalism that you won't find anywhere else in the world.
Bearing in mind, I didn't mix with the Frums.